Riding on Shukla's superlative 117 off 119 deliveries with 16 fours and three sixes, Bengal scored 284 in their first innings to take a 72-run lead. The hosts then pegged UP back to 50 for three with Ashoke Dinda taking two wickets including one that saw Mohammed Kaif's stumps go for a walk.
UP are 22 runs behind and have seven wickets in hand.
Continuing his purple patch, Shukla counter-attacked the UP bowlers to give Bengal a crucial 72-run first innings lead.
For the Bengal skipper, it was his second century this season, and eighth overall, besides a 95 not out in the previous match against Railways.
India discard Rudra Pratap Singh (five for 77) picked his first five-wicket haul this season but it came pretty late as some sloppy wicketkeeping by Ekalavya Dwivedi almost ruined the chances of UP, who should have lead the table.
There was no stopping Shukla who scored with disdain and was at his aggressive best against promising UP pacer Amit Mishra.
There was a further setback for UP as skipper Piyush Chawla could not field again after being hit on his shoulder by a Shukla straight drive in the very first ball that the leg-spinner bowled.
"I had decided to put the pressure back on them. It was my day," Shukla said after the second day's proceedings.
When UP batted, Dinda had Digvijay Singh caught behind before rattling Mohammad Kaif's stumps with a brilliant inswinger to dismiss the former India batsman for a duck.
In the next over, Sourav Sarkar castled night-watchman Mishra for another duck as Bengal ended the day with a lot of optimism.
Brief Scores: Uttar Pradesh 1st Innings 212 and 2nd Innings 50/3 in 17 overs (Dinda 2/36).
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