Binu Kumar (28) and Md Altaf (23) were nabbed by the Crime Branch of the Delhi Police from Delhi Cantonment-Dwarka Road following a tip-off.
A silver Toyota Innova car, allegedly robbed by the duo recently, was recovered from them.
With the arrest, police have claimed to have solved five carjacking cases lodged in Delhi and Gurgaon.
The gang used to target high-end cars after pursuing them for some days.
Describing the modus operandi of the gang, police said, "They used 'gamchas' (cotton towels) and firearms for committing the robberies. They would force the driver of the targeted car to stop and come out of the vehicle, after which they took control by showing the firearm. They would then shift the driver to the rear seats."
In one robbery committed by the gang in March this year, they had hit a Ford Eco Sport car from behind with their stolen car to force the driver to step out of the SUV.
As the driver got out of the car, they robbed him of the vehicle using their modus operandi.
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