The Oscar-winning actress, 38, is also serving the scriptwriter of the project, reported Us magazine.
"It's not a big movie, it's not an action movie. It's the kind of movie we love, but aren't often cast in. It's a very experimental, independent-type film where we get to be actors together and be really raw, open, try things," she said.
Jolie also said that they don't take each other for granted despite being in a relationship for such a long time.
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