"The national hospital was liberated and... 22 foreign mercenaries were killed," the Syrian Democratic Forces (SDF) said.
"Clashes continue with great intensity near the municipal stadium," the other main position still in IS hands, it said.
The advance came a day after the SDF took an infamous roundabout used by the jihadists for public beheadings and crucifixions in Raqa.
The SDF, backed by a US-led coalition, are on the verge of seizing Raqa after having taken around 90 percent of the jihadist group's former de facto Syrian capital.
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