In the first incident, which was claimed by the Islamic State group, a white van sped into a street packed full of tourists in central Barcelona yesterday afternoon, knocking people out of the way and killing 13 in a scene of chaos and horror.
Some eight hours later in Cambrils, a city 120 kilometres south of Barcelona, an Audi A3 car rammed into pedestrians, injuring six civilians -- one of them critical -- and a police officer, authorities said.
Police said they were "working on the hypothesis that the terrorists shot dead in Cambrils are linked to what happened in Barcelona".
Witnesses in Barcelona recounted how bodies were strewn along the famous Las Ramblas boulevard where the driver went on a rampage as other people fled for their lives, screaming in panic.
The carnage in a city hugely popular with tourists from around the world is the latest in a wave of attacks in Europe where vehicles have been used as weapons of terror.
Police announced the arrest of two suspects, identified as a Spaniard and a Moroccan, but said the driver was still on the run.
"We're united in grief," Spanish Prime Minister Mariano Rajoy said in a televised address after rushing to Barcelona, the biggest city in Catalonia, a region in Spain's northeast whose separatist government is defying Madrid with a drive for independence.
"Above all we're united in the firm intention to defeat those who want to take our values and way of life from us."
Belgium said one of its citizens had died in the Las Ramblas assault, while The Hague said three Dutch were injured and a Greek diplomat reported three nationals had been wounded -- a woman and her two children.
Las Ramblas is one of Barcelona's busiest streets, lined with shops and restaurants and normally packed with tourists and street performers until well into the night.
"When it happened I ran out and saw the damage," local shop worker Xavi Perez told AFP.
Tom Gueller, who lives on a road next to Las Ramblas, said he saw the vehicle speeding along the boulevard.
"It wasn't slowing down at all. It was just going straight through the middle of the crowds in the middle of the Ramblas," he told BBC radio.
In Cambrils, meanwhile, Markel Artabe, a 20-year-old restaurant worker, said he was on the seaside promenade when he heard what he initially thought were fireworks, but soon realised were gunshots.
"I saw a foreigner dead with a gunshot in the head. His friends were crying out 'help'. I also saw dead bodies that seemed to be terrorists because they were wearing explosive belts."
It had even seen a surge in tourists as visitors fled other restive sunshine destinations like Tunisia and Egypt.
But it is no stranger to jihadist attacks, having been hit by what is still Europe's deadliest in March 2004, when bombs exploded on commuter trains in Madrid, killing 191 people in an attack claimed by Al Qaeda-inspired extremists.
Police said yesterday that one of the arrested suspects in the Barcelona attack was a Spaniard born in Melilla, a Spanish territory on Morocco's north coast, and the other a Moroccan named as Driss Oukabir.
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