The hosts replied to India's 408-run total with 506 in their first innings with the captain himself scoring a hundred and Mitchell Johnson smacking a quick-fire 88 runs.
"We were six down for 240-odd and Mitchell Johnson came out and took the charge to the Indian bowling," Smith told reporters.
"He took them on and played some terrific cricket. He was positive from ball one. They tried to get stuck in to him and he took them on because it played into his favour. They didn't really have an answer to him after that.
The newly-appointed skipper was humble about his own Test hundred on debut as captain. It was his sixth overall hundred and second of the series so far.
"I said before in the pre-match conference that I wanted to lead from the front. So obviously I am delighted with this hundred as well," said Smith, who became the ninth Australian skipper to score a hundred on captaincy debut.
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