On one of the flattest WACA tracks in recent times, India scored a commanding 309 for three courtesy Rohit's brilliant strokeplay but the target seemed insufficient against the hosts, who relied on centuries by Smith and George Bailey (112) to overhaul the target in 49.2 overs.
Rohit's 163-ball knock was the best by an Indian today while vice-captain Virat Kohli also impressed with a 91-run effort as the duo added 207 runs for the second wicket.
While it was another heartbreaking end to a Rohit century that ended in a losing cause (his T20 hundred and ODI hundred against SA were scored in defeats), Australian skipper Smith again turned out to be India's nemesis pacing his innings to perfection.
Smith's sequence of scores against the 'Men In Blue' across formats reads: 162 not out, 52 not out, 133, 28, 192, 14, 117, 71, 47, 105.
The Indian bowling attack looked completely out of depth as the Smith-Bailey duo never did anything extraordinary but still managed to hammer Umesh Yadav and co with monotonic regularity.
For India, debutant Barinder Sran (3/56) managed to create an impression with early breakthroughs but the other bowlers failed to join the party.
Especially disappointing were India's spin twins Ravichandran Ashwin (2/68 in 9 overs) and Ravindra Jadeja (0/61 in 9 overs) looked far from penetrative.
They could hardly extract any turn and were played with consummate ease by the Aussie captain, whose footwork was exemplary.
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