"Ibrahim al-Barakat was arrested early on Sunday and is accused of being a religious jurist for Daesh in the northern city of Tripoli," the security official told AFP, using the Arabic acronym for IS.
Barakat, who is in his 40s, was arrested while trying to flee northern Lebanon to Turkey using a fake passport.
He is accused of recruiting young men from Tripoli to fight with IS in Syria and Iraq and of attacking Lebanese army units in the Sunni-majority city last year.
Sunni gunmen in the city have often also clashed with the army.
In October 2014, 11 soldiers were killed when clashes erupted following the arrest of a Lebanese man accused of recruiting fighters for jihadist rebel groups in Syria.
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