Brunhilde Pomsel died on January 27 in a care home in the southern city of Munich, said Christian Kroenes, who conducted extensive interviews with her for his 2016 film "A German Life".
Pomsel, who worked for Goebbels as a secretary, typist and stenographer from 1942-45, had insisted she had no idea of the Holocaust that claimed the lives of six million Jews while it was happening.
"We knew nothing," she said in the film.
As one of half a dozen secretaries in Goebbels' office, Pomsel was among the last eyewitnesses to the inner circle of top Nazis.
In "A German Life", she insisted she felt no guilt and also said: "I could not put up resistance -- I was too much of a coward."
She told AFP last year that she had once cheered on Hitler, in 1933, adding "we didn't know then what lay ahead".
She spoke of the final days in Hitler's bunker, saying a lot of alcohol was drunk because the Nazi chiefs had to "numb themselves".
From 1950 she worked for a German public broadcaster, for 20 years, but kept silent about her war-time job until she gave a newspaper interview in 2011.
She opened up at great length in the 2016 film, which its makers said aimed to force viewers to ask themselves what they would have done, and whether they would have had the courage to resist the Nazi machine.
In the black-and-white film, extreme close-up shots of Pomsel recalling her time with Goebbels are interspersed with archival footage of Nazi horror, including of naked Jewish corpses and mass graves.
"I wouldn't see myself as guilty," she said, "unless you end up blaming the entire German population".
She said that "since I have a clear conscience for myself, I do not see why I should not talk about it".
She said the point of the film was "for future generations to be informed about all these things. There are ever fewer eyewitnesses left. So I agreed."
She described Goebbels as well groomed and polite, and "an excellent actor," who during public speeches turned into a "raging dwarf ... Unrecognisable"
Asked about rising right-wing populism in Europe now, she said she found it "horrific, just horrific".
Filmmaker Kroenes confirmed to AFP that she died on January 27 in the old people's home but had remained mentally alert until her death.
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