Jadeja achieved the feat while bowling in Sri Lanka's first innings on day three of the second Test.
Ashwin had reached the milestone in 29 Tests while Jadeja managed it in 32 games.
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He also became the fastest Indian left-arm spinner to reach 150 wickets, ahead of Vinoo Mankad (40 Tests), Bishan Bedi (41 Tests) and Ravi Shastri (78 Tests).
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