Singh (7/42) added six more to his overnight tally and returned with 14 maidens from his 27 overs to bring Kerala's downfall from being 290/2 losing last five wickets for eight runs.
In reply, Goa were 169/6 with V Vinod Kumar (3/33) rocking their middle-order with two wickets in three balls.
Sanju Samson edged Singh behind the stumps to become the first victim of the day in the third over before Saurabh Bandekar (2/77) joined him at the other end.
Goa 1st Innings 169/6; 60 overs (Vinod Kumar 3/33).
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