Microscopic analysis of the meteorite also suggests that liquid water was present on Mars more recently than believed.
The Lafayette meteorite was discovered in Indiana, US in 1931, having plummeted to Earth about 3,000 years ago.
It formed in the Red Planet's crust about 1.3 billion years ago and was ejected from the surface by a massive impact.
The rock shows signs of carbonation - where minerals absorb CO2 in a reaction with water, 'BBC News' reported.
They found that silicate minerals, such as olivine and feldspar, had interacted with CO2-rich liquid water to form siderite crystals.
The team said their discovery suggests liquid water was present on Mars more recently than some had thought.
They also said it represents the first direct evidence for carbonation on the Red Planet - and ties in with the discovery of carbonates by NASA's Curiosity Mars rover.
"Carbonation could be the main force that turned Mars to stone," said lead author Dr Tim Tomkinson, of SUERC.
The loss of its carbon dioxide cloak is likely to have caused Mars to cool. So understanding how the CO2 was removed "could provide vital clues to how we can limit the accumulation of carbon dioxide in the Earth's atmosphere and so reduce climate change," said Tomkinson.
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