Prime Minister Mariano Rajoy yesterday sought to reassure Spaniards, saying in an interview published in the daily El Pais at the end of the day of protest that if an independence declaration is made it won't have any effect.
"The government will ensure that any declaration of independence will lead to nothing," he told El Pais.
He also urged moderate Catalan nationalists to distance themselves from the "radicals" in the separatist camp who are pushing hardest for an independence move.
"I am sad to see the state in which we find our country and the mediocrity of our government," said Marte Muro, 67, at the rally in Madrid which drew several thousand people.
In Barcelona thousands packed Sant Jaume square in front of city hall as tension reigned with no solution in sight to Spain's worst political crisis in a generation.
They held up signs with the word "parlem" -- Catalan for "let's talk" -- and waved white handkerchiefs but not flags.
But in Madrid, parallel to the "Let's Talk" march, some 50,000 people according to Spain's central government gathered in Colon Square beneath an enormous Spanish flag for a "patriotic" march organised by activists to defend unity.
"Rajoy, you asshole, defend the nation!" chanted one group of demonstrators as they marched into Colon Square waving Spanish flags as well as one bearing the Franco-era black eagle.
Separate from that group, Octavi Puig, a retired Catalan who lives in Madrid, said he came to the protest because he did not want a "Berlin wall" to separate him from the graves of his loved ones and his family in Catalonia.
The rallies followed days of soaring tensions after police cracked down on voters during a banned October 1 Catalan independence referendum, prompting separatist leaders to warn they would unilaterally declare independence in days.
Tentative signs emerged Friday that the two sides may be seeking to defuse the crisis after Madrid offered a first apology to Catalans injured by police during the vote.
But uncertainty still haunts the country as Catalan leaders have not backed off from plans to declare the region independent.
And Catalan leader Carles Puigdemont said he has had "no contact" with the central government to try to resolve the crisis.
Rajoy has rejected calls for mediation in a dispute that has drawn cries of concern all over Spain, and even from Barcelona and Real Madrid footballers.
The crisis has raised fears of unrest in the northeastern region, a tourist-friendly area of 7.5 million people that accounts for a fifth of Spain's economy.
Businesses and the government have kept up economic pressure on Catalonia, with several big companies announcing moves to shift their headquarters to other parts of Spain.
It remains unclear what he plans to say, although some separatist leaders hope he will use the opportunity to make a declaration of independence.
If Catalonia declares independence, Spain could respond by suspending the region's existing autonomous status and imposing direct rule from Madrid.
The Catalan government on Friday published final results from the referendum indicating that 90 percent of voters backed the idea of breaking away from Spain.
Turnout was 43 percent. The vote was not held according to regular electoral standards, without regular voter lists or observers.
With its own language and cultural traditions, demands for independence in Catalonia date back centuries but have surged during recent years of economic crisis.
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