Fry, 56, will voice an aristocratic deer called Lord Stag in 'Driftwood Bay', reported BBC online.
The show, which will air in May, is about a young girl who creates an imaginary world from treasures she finds on the beach.
Horrocks will play Wee Rabbit while Mullan, best known for hard-hitting dramas, will be Salty Dog the sailor.
"I've never done any voice work on animation so I thought this was a nice chance to do something that my children can actually see me in for a change!," Mullan said.
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