Police announced that a 30-year-old man had been arrested in east London following the attack in the capital on Saturday, which left seven confirmed dead and 48 injured.
They also said a body had been recovered from the Thames in the search for a missing Frenchman.
Conservative Prime Minister Theresa May and Labour leader Jeremy Corbyn scheduled eve-of-polling whistlestop campaigns, targeting urban areas whose vote could be crucial.
May aimed at the high-population English Midlands in her final dash, while Corbyn was to attend six rallies in England, Scotland and Wales, stretching from Glasgow to London, in a gruelling last-day marathon.
But the political ground began to shift under her feet, moving from EU membership -- May's strongest card -- to domestic policy and her own record on security, both of them favouring Corbyn.
Opinion polls -- hampered by a poor reputation for reliability -- predict a May win. But according to polling methodology, victory could range from around 50 seats, to a small majority or even no majority at all.
"Get those negotiations wrong and the consequences will be dire," May said today.
Corbyn made an eve-of-voting pitch on the National Health Service (NHS), a beloved institution.
"The Conservatives have spent the last seven years running down our NHS, our proudest national institution. Our NHS cannot afford five more years of underfunding, understaffing and privatisation," he said.
Despite being seen as an unlikely leader -- one who has faced off a rebellion by his own MPs -- Corbyn has gained momentum during the election campaign and regularly attracts big crowds to his rallies.
The pledge hit the party's core supporters and May was forced to backtrack on capping the costs, prompting further criticism that she was unreliable.
Corbyn then found a valuable seam in attacking May on security, an area where the Conservatives traditionally are far stronger than Labour in voters' minds.
A string of terror attacks have occurred since May became prime minister last July, and she was interior minister for six years before she rose to the top job.
"The expectations of the opinion polls are extremely divergent," said John Curtice, a professor of politics at Strathclyde University in Scotland, who said the outcome could hinge on the turnout among young voters, believed to be overwhelmingly pro-Labour.
University of London professor Eric Kaufmann agreed, but noted that traditionally turnout among young people in British elections was low.
"There's no obvious reason why that would rebound," he said. "I'm sort of with the general polls which suggest that the Tories will increase their majority by around 25 seats... a good majority, not as much as it looked it could have been at one point, but I think it's pretty solid."
Questions are also being raised about the vaunted image of Britain's security services. Three terror attacks have taken place since March, leaving 34 dead and around 200 injured, and all involved assailants who were known to the authorities.
In the most recent attack, seven people were killed on Saturday when three men aboard a hired van ploughed into pedestrians on London Bridge and went on a stabbing spree before being shot by police.
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