Officials said Shah was arrested under the provisions of the Prevention of Money Laundering Act (PMLA) as "he was not cooperating in the investigation".
They said Shah was questioned by the investigating officer of the case here today after which he was placed under arrest.
"Shah will be produced in a special anti-money laundering court here tomorrow," an ED official said.
Shah was also named in the first charge sheet filed by the ED in this case last year.
Officials had said the central probe agency, at a recent review meeting, had informed the Finance Ministry that it was preparing to initiate fresh action for attachment of assets against the accused and would also question a number of them based on inputs gathered by its investigators till now.
The agency had filed a 20,000-page charge sheet against NSEL and 67 others in a Mumbai court in March last year, explaining NSEL funds were laundered and "illegally plouged into purchase of private properties".
ED had registered a criminal case under the PMLA in 2013 to probe the case, along with the Economic Offences Wing (EOW) of Mumbai police.
After a high-level meeting, chaired by Economic Affairs Secretary Shaktikanta Das, last month, the Centre also directed the Maharashtra government to expedite the resolution of the case by quickly auctioning assets worth Rs 6,116 crore attached so far and refund investors at the earliest.
NSEL's payment troubles started after it was ordered by regulator Forward Markets Commission (FMC) in July 2013 to suspend spot trade in most of its contracts due to suspected trading violations.
Financial Technologies India Ltd (FTIL) blamed NSEL executives and the trading parties for the default. There were 24 members who defaulted payment to about 13,000 investors.
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