The 24-year-old had clocked 9.99 sec at Rome's Diamond League last Thursday, enough to qualify for the August 5-21 Rio Games.
He became co-holder of the European 100m record on July 4, 2015 in Paris when he matched the mark set by Portugal's Francis Obikwelu at the 2004 Athens Olympics.
"I thought I'd put in a big time today. I'm really satisfied with that," said Vicault.
His time is the quickest 100m run anywhere in the world this year, ahead of Qatari Femi Ogunode (9.91), veteran Kim Collins (9.93) and Justin Gatlin (also 9.93).
The six-time Olympic gold medallist owns the 100m world record at 9.58.
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