His comments came after Russian Foreign Minister Sergey Lavrov acknowledged there was no "common vision" between the two nations over the crisis in Ukraine.
The vote in Crimea Ukraine's strategic Black Sea peninsula of 2 million people is widely expected to back secession and possibly lead to annexation with Russia at some point. The new government in Kiev believes the vote is illegal, but Moscow says it does not recognize the new government as legitimate.
Kerry said today he had put forward several ideas on how to respect Ukraine's sovereignty and address Russian concerns in the talks in London, but that Lavrov made clear that Russian President Vladimir Putin would not take any decisions until after Sunday's vote.
Lavrov today reaffirmed that Russia will "respect the results of the referendum" in Crimea and said sanctions would harm relations.
European and US leaders have repeatedly urged Moscow to pull back its troops in Crimea and stop encouraging local militias there who are hyping the vote as a choice between re-establishing generations of ties with Russia or returning to echoes of fascism from Ukraine's World War II era, when some residents cooperated with Nazi occupiers.
The showdown between Russia and the West has been cast as a struggle for the future of Ukraine, a country with a size and population similar to France. Much of western Ukraine favors ties with the EU, while many in eastern Ukraine have closer economic and traditional ties to Russia. Putin has worked for months to press Ukraine back into Russia's political and economic orbit.
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