Khan resigned from the TDP membership and also its politburo of which he was a member, party sources said.
He faxed his resignation letter to the TDP headquarters.
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Khan had unsuccessfully contested the Lok Sabha election from Hyderabad as TDP candidate in 2009.
His son Amer Ali Khan recently joined the YSR Congress and is seeking to contest the April 30 election from Secunderabad parliamentary constituency.
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