Moreover, improved rains and falling global crude prices, which boosted hopes of a rate cut by the Reserve Bank next month, too accelerated buying, traders said.
Sun Pharma's shares today recovered on value-buying and surged 3.35 per cent to Rs 833.05 after tumbling 15 per cent in yesterday's trade.
Meanwhile, a Rajya Sabha Select Committee endorsed almost all the provisions in the landmark bill on GST, while also agreeing to demands of parties like TMC for a five-year compensation to states.
The gauge had lost 281.17 points in the last two days.
The 50-share NSE Nifty after regaining the 8,600-level, scaled session's high of 8,643.90 before settling 104.05 points or 1.22 per cent higher at 8,633.50, its highest closing since April 16.
Among Sensex gainers, RIL topped the list by surging 4.26 per cent on buying by participants on hopes of a strong earnings to be released on Friday.
Among sectoral indices, BSE oil&gas index gained the most by soaring 2.36 per cent, followed by Banking 1.45 per cent.
ICICI Bank rose 1.80 per cent, SBI gained 1.67 per cent, HDFC Bank 1.43 per cent and Axis bank 0.81 per cent.
In commodities, brent oil has now fallen nearly 10 per cent in July. India imports more than 75 per cent of its crude. Brent crude for September delivery was trading lower at USD 56.51 a barrel.
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