"I do not think another extension is in the interest of anyone, as I do not believe this extension was either necessary or useful," Zarif told a global security conference, meeting in the southern German city of Munich.
"In my view extension is not useful, not conducive to an agreement, and all my energy and focus and that of my colleagues and I'm sure my negotiating partners .... Are all focused on reaching an agreement as early as possible."
Kerry and Zarif held a second round of talks here today, meeting for about 90 minutes as they try to hammer out a political accord to rein in Iran's atomic ambitions ahead of a March 31 deadline. Kerry was due to fly back to Washington later in the day.
Few details of the tough negotiations have leaked, but world powers are trying to ensure that Iran's pathways to developing a nuclear weapon are cut off, in return for a gradual easing of international sanctions which have crippled Iran's economy.
Zarif refused to publicly discuss the details of the accord, but said "we are engaged in a very serious discussion."
"We believe it is in our interest to show the world that our programme is exclusively peaceful."
But he also said: "I don't think if we don't have an agreement it will be the end of the world. We try, we fail."
He took issue with the idea of a gradual phasing out of the sanctions, saying there was nothing in the November 2013 interim accord saying that the punishing measures would be removed in a step-by-step process.
The Islamic Republic has long denied accusations that it is seeking to develop an atomic bomb, arguing that its nuclear programme is solely for its civilian energy needs.
But scepticism is mounting about whether a deal is possible, after two deadlines for a comprehensive agreement were missed.
Iran and the group known as the P5+1 -- Britain, China, France, Germany, Russia and the US -- now want to conclude a political agreement by late March, with a final deadline pinning down the technical details by the end of June.
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