Using an icebox-like instrument nicknamed Himalaya, the researchers show that fluffy ice on the surface of a comet would crystalise and harden as the comet heads toward the Sun and warms up.
As the water-ice crystals form, becoming denser and more ordered, other molecules containing carbon would be expelled to the comet's surface. The result is a crunchy comet crust sprinkled with organic dust.
"A comet is like deep fried ice cream," said Murthy Gudipati of NASA's Jet Propulsion Laboratory in Pasadena, California, corresponding author of the study in The Journal of Physical Chemistry.
In the new study, researchers put together a model of crystallising comet crust. The experiments began with amorphous, or porous, ice - the proposed composition of the chilliest of comets and icy moons.
In this state, water vapour molecules are flash-frozen at extremely cold temperatures of around minus 243 degrees Celsius.
Disorderly states are preserved: Water molecules are haphazardly mixed with other molecules, such as the organics, and remain frozen in that state. Amorphous ice is like cotton candy, explained Gudipati: light and fluffy and filled with pockets of space.
The ice had been infused with a type of organics, called polycyclic aromatic hydrocarbons, or PAHs, which are seen everywhere in deep space.
"The PAHs stuck together and were expelled from the ice host as it crystallised," said lead study author Antti Lignell, at the California Institute of Technology in Pasadena, who formerly worked with Gudipati at JPL.
"This may be the first observation of molecules clustering together due to a phase transition of ice, and this certainly has many important consequences for the chemistry and physics of ice," said Lignell.
"What we saw in the lab - a crystalline comet crust with organics on top - matches what has been suggested from observations in space," said Gudipati.
"Deep fried ice cream is really the perfect analogy, because the interior of the comets should still be very cold and contain the more porous, amorphous ice," he said.
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